As a heads up, if you do decide to go the big-terrifying-outrunner route, all of the Alien Power Systems and Epowerhobby stuff is just made by FRCHobby in China. They have an Alibaba store, so you can just get what you want directly from them.
I don't have an actual answer as far as if an opensource controller will run it well, and most of what I know involves the 120mm outrunners, but your biggest concern for controller selection is going to be erpm (because of the hilariously high pole count) and current levels.
For the 120100's that I have (I'm going to run two of them in a motorcycle), they're 50kV motors with 28 poles rated at 25kW each, and I would need 70,000erpm in order to get 5,000 rpm out of the motor. My controllers are pretty small (Kelly KLS7230S's, 120A cont/300A max), and in a few days once my usb-serial converter shows up I'll have a lot more info for you about how well the controllers can run one of these. Since my pack comes off the charger at 84 volts, we're looking at a maximum of 4200rpm, which will still be more than enough for highway speeds with good acceleration, if the controllers play nice.
With a 27kV motor, you probably aren't going to be looking to spin it higher than 2500rpm (~92 volts) anyways, so you'd be pretty okay with a ~40,000erpm controller like one of the big APT's I linked below even if it has 32 poles. With up to 600A of phase current, you could probably move a motorcycle pretty well with one of these.
http://www.cnqsmotor.com/en/article...V 96V 8kW PM Motor Driver Controller/332.html
I'm just about done sourcing parts for my build, and I kind of wish I'd gone higher voltage rather than high current 20s, though. Running a bunch of 1/0 wire is going to be a bit of a pain.