To be frankly honest with you, I'm more a mini geared hub kind of guy, with only some basic experience in direct drive motors, so there are plenty here who could give you better advice than I can, but since it's been about 4 hours since you posted and nobody has, I'll give you a start.
1. LiPo - I do have experience here. Don't forget that 18S2P is 66.6v NOMINAL. Hot off the charger, it's 75.6v. Make sure your "60v" controller can handle 75.6v. Or preferable one or two volts higher, since you can't trust chargers and temperature to be consistent.
2. I've never owned a HS3540. I know that there are plenty using them at 3000w, but your controller and battery pack set up has the potential to push out over 6000w on full charge. A quick google only showed one recommendation for current limiting - 40A, but it didn't say at what voltage.
3. If you get anywhere near that, be absolutely sure you have the other safety aspects locked down first. I'd be thinking front and rear hydraulic discs. Also, are you using torque arms? Many thought I was crazy for not using torque arms on 1kw. Anything above that, and you'd be crazy, especially if you're fitting it to a front fork. Have you thought about the capability of the bike to handle the kinds of speeds you're likely to get? The HS3540 has a target speed of 40km @36v. In theory, if you don't melt the entire setup, you should be expecting 80km/h. Front and rear suspension would be a must, and you'd want to make sure you have a very good quality frame, and not something cheap that's going to disintegrate the first pothole you hit at 50km/h.
IMHO, I would get a programmable controller first, and limit myself to 40A first. The Stealth Fighter uses that as a tried and true motor combo. Take it easy and after 100km, check your bike for any signs of cracking excessive wear or damage. Only then would I start tweaking it up from there.
Oh - and with the current that you could potentially put out, if you run it at full throttle (80A), expect around about 7.5 minutes of battery life. Another reason to cut down the power until you have more juice.
Again, reminder that I have no experience in with this motor. My advice is just to take it easy, your setup sounds very dangerous for a second build.